The cold open for The Nth Degree (I think?) where he and Beverly are doing a production of something, it keeps showing the audience. Everyone is smiling and having a good time... Except Data, who has the look of someone who just smelled a fart, which sours more when he looks around the room to see everyone else's reaction and I just know he is thinking "how the hell are they enjoying this absolute shit show? I could act circles around Broccoli!"
Gets me every time. 💀